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Wei, Zitang; Wang, Kang; Zhao, Wenchao; Gao, Yao; Hu, Qixuan; Chen, Ke; Dou, Letian (, Chemical Communications)A selenophene-containing conjugated organic ligand, 2-(4′-methyl-5′-(5-(3-methylthiophen-2-yl)selenophen-2-yl)-[2,2′-bithiophen]-5-yl)ethan-1-aminium (STm), was synthesized and incorporated into a Sn( ii )-based two-dimensional perovskite, (STm) 2 SnI 4 . The band offset between the perovskite and ligand can be fine-tuned by introducing the STm ligand. Both field-effect transistor and light-emitting diode devices based on (STm) 2 SnI 4 films exhibit high performance and enhanced operational stability.more » « less
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Zhang, Shuyang; Pink, Maren; Junghoefer, Tobias; Zhao, Wenchao; Hsu, Sheng-Ning; Rajca, Suchada; Calzolari, Arrigo; Boudouris, Bryan W.; Casu, Maria Benedetta; Rajca, Andrzej (, Journal of the American Chemical Society)
